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Titolo:
Concise synthesis of the C3-C14-fragment of the antitumor agent laulimalide. Application of Jacobsen's HKR reaction
Autore:
Dorling, EK; Ohler, E; Mantoulidis, A; Mulzer, J;
Indirizzi:
Univ Vienna, Inst Organ Chem, A-1090 Vienna, Austria Univ Vienna Vienna Austria A-1090 nst Organ Chem, A-1090 Vienna, Austria
Titolo Testata:
SYNLETT
fascicolo: 7, , anno: 2001,
pagine: 1105 - 1108
SICI:
0936-5214(200107):7<1105:CSOTCO>2.0.ZU;2-D
Fonte:
ISI
Lingua:
ENG
Soggetto:
ENANTIOSELECTIVE SYNTHESIS; MACROLIDE LAULIMALIDE; SEGMENT; ALDEHYDES; FRAGMENT; TAXOL;
Keywords:
antitumor agents; epoxides; Jacobsen's HKR reaction; Eschenmoser methylenation;
Tipo documento:
Article
Natura:
Periodico
Settore Disciplinare:
Physical, Chemical & Earth Sciences
Citazioni:
26
Recensione:
Indirizzi per estratti:
Indirizzo: Mulzer, J Univ Vienna, Inst Organ Chem, Wahringerstr 38, A-1090 Vienna, Austria Univ Vienna Wahringerstr 38 Vienna Austria A-1090 enna, Austria
Citazione:
E.K. Dorling et al., "Concise synthesis of the C3-C14-fragment of the antitumor agent laulimalide. Application of Jacobsen's HKR reaction", SYNLETT, (7), 2001, pp. 1105-1108

Abstract

Bromide 3, which represents an appropriately functionalized C3-C14-fragment of the antitumor agent laulimalide (1) has been synthesized from (-)-citronellal (4) in an overall yield of ca. 17% (12 isolated intermediates). At a very early stage, the synthesis makes use of Jacobsen's HKR reaction to produce epoxide 8 in diastereomerically pure form.

ASDD Area Sistemi Dipartimentali e Documentali, Università di Bologna, Catalogo delle riviste ed altri periodici
Documento generato il 26/05/13 alle ore 05:09:33